My set of allen keys aren't marked with sizes but did a quick measurement with an old imperial micrometer (0.156"), multiplied by 25.4 and I'm pretty sure it's 4mm.
That's an old grundfos 15-50, yours may be different.
there is no best size to take the head off, there is only 1 size that fits, and it is in metric.
don't bother checking if the impeller fell off, it didn't
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