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"Which method you are suggesting".....what a strange question to ask..A genuine question, why refer to "increasing the CO2%" without saying which method you are suggesting.
The percentage of CO2 in the exhaust gas can be increased by
EITHER
increasing the gas flow rate and leaving air flow rate un-changed
OR
reducing the air flow rate and leaving the gas flow rate unchanged
Do you know what the effects would be when increasing CO2%?